Thursday, December 31, 2009

Luminescence properties of double-perovskite Sr2Ca1−2xEuxNaxMoO6 red-emitting phosphors prepared by the citric acid-assisted sol–gel method

Luminescence properties of double-perovskite Sr2Ca1−2xEuxNaxMoO6 red-emitting phosphors prepared by the citric acid-assisted sol–gel method: "

Abstract  Double-perovskite Sr2Ca1−2x
Eu
x
Na
x
MoO6 red-emitting phosphors were prepared by the citric acid-assisted sol–gel method, and their luminescence properties were investigated
as a function of sintering temperature and Eu3+-doping concentration. B-site substituted Sr2Ca0.8Eu0.1Na0.1MoO6 phosphor, in which Na+ ions act as charge compensators, was selected to study the thermal behavior, phase structure, microstructure, and photoluminescence
property under different sintering temperatures. The photoluminescence studies on Sr2Ca1−2x
Eu
x
Na
x
MoO6 (x = 0.02, 0.05, 0.10, 0.15, 0.2) show that a dominant red emission line at around 594 nm, which is due to the Eu3+ magnetic dipole transition of 5D07F1, is observed under different Eu3+ excitations (396 and 412 nm). Further, Eu3+ dopant content dependent emission spectra investigations of Sr2Ca1−2x
Eu
x
Na
x
MoO6 phosphors indicates that, when the Eu3+ concentrations x = 0.05, there are minimum differences between the emission intensity of 5D07F1 transition at 594 nm and that of 5D07F2 transition at 615 nm. With increasing Eu3+ concentration, the variation of the emission intensities between the two transitions keep nearly invariable and Sr2Ca0.8Eu0.1Na0.1MoO6 phosphor has the strongest red emission in this series.


  • Content Type Journal Article
  • DOI 10.1007/s10853-009-4123-2
  • Authors

    • Zhiguo Xia, China University of Geosciences School of Materials Sciences and Technology Beijing 100083 China
    • Jianfeng Sun, Beijing Technology and Business University College of Chemistry and Environmental Engineering Beijing 100048 China
    • Haiyan Du, Beijing Technology and Business University College of Chemistry and Environmental Engineering Beijing 100048 China
    • Daimei Chen, China University of Geosciences School of Materials Sciences and Technology Beijing 100083 China
    • Jiayue Sun, Beijing Technology and Business University College of Chemistry and Environmental Engineering Beijing 100048 China


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